Just for curosity, that guy with the crank, would it happen to be Hardy Prentice, I used to race with him at the runoffs back in the 80s, he had the fastest TR3 race car, I'm pretty sure he won a championship with it in the early 90s, if it is Hardy, he real good people, and you can trust whatever he tells you.
Tuffriting and nitriting are surface hardening treatments, they normally impregnate the crank's metal about .030" and are use to make for good crank journal wear. Most all factory cranks had some sort of surface hardening process done to them, and it is retained down to .020/.020, if you have to go to .030/.30, then you compromised the hardening and there are companies they will reharden the crank for you, Ion nitriting is popular these days because it's less work, David Anton at APT offers this, than the traditional salt bath type nitriting, where the crank has to be restraighten after the process, also the journals have to re polished as well. The radius that is referred to is done during crank grinding, it is normal, and comes from the factory that way, but they are many crank grnders that butcher cranks, so having a good crank grinder who put the proper filet radius back into the journal is key to crankshaft life, without it, a strees riser is created and cranks crack at the journal because of non existent filet radiuses. I'd say 80% of the cracked crankshafts I have seen in my life were a result of the crank being ground undersize from standard by a shotty crank grinding job where the filet radius was not kept proper.
Oh and that head combustion chamber photo, looks like a recessed exhaust valve from where I'm sitting, and that head does not have hardened exhaust seat inserts, so time to think about getting that done as well.